Leonard Nimoy, as the character Dr Spock in Star Trek can do it and of course Sean Connery too....but for most of us its impossible. I can raise both eyebrows at once, but not one at the time. Raising or cocking the eyebrow may be an evolutionary trait: baboons, mandrills and cebus monkeys are said to raise their eyebrows as a threat gesture.

This dictionary makes entertaining reading....everything
From Adam's-Apple-Jump to Zygomatic Smile
The Nonverbal Dictionary